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Lithiation and Delithiation Reactions of Binary Silicide Electrodes in an Ionic Liquid Electrolyte as Novel Anodes for Lithium‐Ion Batteries
https://repository.lib.tottori-u.ac.jp/records/7134
https://repository.lib.tottori-u.ac.jp/records/7134efc0c4b4-ee90-4c34-a1f1-9f27fd8522e3
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<td class="multiple-line">Lithiation and Delithiation Reactions of Binary Silicide Electrodes in an Ionic Liquid Electrolyte as Novel Anodes for Lithium‐Ion Batteries</td>
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<th scope="row" colspan="5" style="border: 0px !important;">主題</th>
<td class="multiple-line">lithium-ion batteries</td>
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<th scope="row" colspan="5" style="border: 0px !important;">主題</th>
<td class="multiple-line">silicide</td>
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<td class="multiple-line">ionic liquid electrolyte</td>
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<td class="multiple-line">gas deposition</td>
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<td class="multiple-line">soft X-ray emission spectroscopy</td>
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<td class="multiple-line">lithium-ion batteries</td>
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<th scope="row" colspan="5" style="border: 0px !important;">主題</th>
<td class="multiple-line">silicide</td>
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<th scope="row" colspan="5" style="border: 0px !important;">主題</th>
<td class="multiple-line">ionic liquid electrolyte</td>
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<td class="multiple-line">gas deposition</td>
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<td class="multiple-line">soft X-ray emission spectroscopy</td>
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<td class="multiple-line">journal article</td>
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<th scope="row" colspan="5" style="border: 0px !important;">値</th>
<td class="multiple-line">Department of Chemistry and Biotechnology, Graduate School of Enginnering, Tottori University / Center for Research on Green Sustainable Chemistry, Tottori University / Global Research Center for Environment and Energy based on Nanomaterials Science, National Institute for Materials Science</td>
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<td class="multiple-line">Department of Chemistry and Biotechnology, Graduate School of Enginnering, Tottori University / Center for Research on Green Sustainable Chemistry, Tottori University / Global Research Center for Environment and Energy based on Nanomaterials Science, National Institute for Materials Science</td>
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<td class="multiple-line">Graduate School of Sustainability Science, Tottori University / Center for Research on Green Sustainable Chemistry, Tottori University / Global Research Center for Environment and Energy based on Nanomaterials Science, National Institute for Materials Science</td>
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<td class="multiple-line">Department of Chemistry and Biotechnology, Graduate School of Enginnering, Tottori University / Center for Research on Green Sustainable Chemistry, Tottori University / Global Research Center for Environment and Energy based on Nanomaterials Science, National Institute for Materials Science</td>
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<td class="multiple-line">We investigated the lithiation and delithiation properties of pure binary silicide electrodes in an ionic liquid electrolyte as novel anodes for lithium‐ion batteries. Some electrodes maintain a high reversible capacity in the electrolyte, whereas they show a poor cycling performance in an organic electrolyte. The superior performance results from the high affinity for the transition metal that composes the silicide with Li. Based on reaction behavior analysis, the crystal structure of silicide is maintained during the cycling, and phase separation does not occur. The ionic liquid electrolyte suppresses the formation of cracks and exfoliation of the silicide layer from a substrate. In addition, a surface film formed on the silicide electrode through the reductive decomposition of the electrolyte has different components than that on a Si electrode, even in the same ionic liquid electrolyte. Soft X‐ray emission spectroscopy demonstrates that the pure silicide itself reacts with Li. The obtained results will provide significant insights into novel alloy‐based anode materials for lithium‐ion batteries.</td>
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<td class="multiple-line">Wiley-VCH Verlag GmbH & Co. KGaA.</td>
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<th scope="row" colspan="5" style="border: 0px !important;">収録物識別子</th>
<td class="multiple-line">21960216</td>
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<td class="multiple-line">10.1002/celc.201801088</td>
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<td class="multiple-line">© 2018 The Authors. Published by Wiley-VCH Verlag GmbH & Co. KGaA. This is an open access article under the terms of the Creative Commons Attribution License, which permits use, distribution and reproduction in any medium, provided the original work is pr</td>
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<td class="multiple-line">This research was published by Wiley: DOMI, Yasuhiro, et al. Lithiation and Delithiation Reactions of Binary Silicide Electrodes in an Ionic Liquid Electrolyte as Novel Anodes for Lithium‐Ion Batteries. ChemElectroChem, 2019, 6.2: 581-589. https://doi.org</td>
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<td><a href="https://onlinelibrary.wiley.com/doi/full/10.1002/celc.201801088" target='_blank'>https://onlinelibrary.wiley.com/doi/full/10.1002/celc.201801088</a></td>
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<td><a href="https://onlinelibrary.wiley.com/doi/full/10.1002/celc.201801088" target='_blank'>https://onlinelibrary.wiley.com/doi/full/10.1002/celc.201801088</a></td>
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<td class="multiple-line">VoR</td>
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Item type | 学術雑誌論文 / Journal Article(1) | |||||||||||||
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Domi, Yasuhiro
× Domi, Yasuhiro
× Usui, Hiroyuki
× Takaishi, Rena
× Sakaguchi, Hiroki
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ChemElectroChem en : ChemElectroChem 巻 6, 号 2, p. 581-589, 発行日 2018-10-12 |
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Domi, Yasuhiro, Usui, Hiroyuki, Takaishi, Rena, Sakaguchi, Hiroki, 2018, Lithiation and Delithiation Reactions of Binary Silicide Electrodes in an Ionic Liquid Electrolyte as Novel Anodes for Lithium‐Ion Batteries: Wiley-VCH Verlag GmbH & Co. KGaA., 581–589 p.
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